Like 150EH said, it's all about CO2 diffusion, surface agitation, and good flow to distribute the dissolved CO2.
Google Amano's ADA tanks. They're all open top.
EDIT: How much of a pH drop are you getting? In my tank (48"x18"x18"), my pH during the lights on drop all the way to 6-6.2. The tank water I took out and let sit for 24 hours test out to pH 7.4. While pH drop isn't the best way to measure dissolved CO2, it's a good starting line.