I've kept a few cardinals with a betta in a 5.5gal before, didn't have any problems, just changed 10% of the water weekly and everything was good for several years (was a tank at work so I took it down after I quit that job and we moved).
I'd say the 5gal sounds rather full ATM though; you could add the betta but will probably need to change more like 50% a week (2x 25% weekly would be better) b/c that would definitely be a high bioload. What kind of filter do you have on there?
I wouldn't be surprised if the molly does decide to take nips out of the betta's fins in the other tank, though.
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